Sylar is a character in Heroes though, and nothing else major seems to be associated with that name, so a Pokemon character having that name would be pretty off I think considering how he was the "bad guy" and all.
How about the names being taken from a word? Like how Nate/Rosa was from "resonate" (along with their Japanese names). I'm really bad at making up names myself though, but a spontaneous thought was the nucleobases.



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