I like the Jigglypuff in the Sound Test, and I also like the Musharna that appears when you connect to Wi-fi to tuck in a Pokemon for Pokemon Dream World.
I also like the Spiritomb from Pokemon Ranger: Shadows of Almia.
And mah Shinx.
I'm a full time Pokemon Breeder! But please visit, I really do appreciate the help.
Not sure if this counts or not but...
The Darkrai and the Lickilicky from the movie Darkrai Rises, Richie's Pikachu and Jessie's Wobbuffet.